Direct fused deposition modeling 4D printing and programming of thermoresponsive shape memory polymers with autonomous 2D‐to‐3D shape transformations

Hu, G. and Bodaghi, M. ORCID: 0000-0002-0707-944X, 2023. Direct fused deposition modeling 4D printing and programming of thermoresponsive shape memory polymers with autonomous 2D‐to‐3D shape transformations. Advanced Engineering Materials: 2300334. ISSN 1438-1656

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Abstract

Herein, direct 4D printing of thermoresponsive shape memory polymers (SMPs) by the fused deposition modeling (FDM) method that enables programing of 2D objects during printing for autonomous 2D-to-3D shape transformations via simply heating is focused on. The programming process during printing is investigated through designs and experiments. The capability of programming SMPs during printing is illustrated by prestrain and bending capabilities, which are highly related to printing settings, such as nozzle temperature, print speed, layer height, infill patterns, and ratio of active parts in a bilayer structure. A nearly linear relationship for prestrain and bending parameters is experimentally revealed for different printing factors. Quantitative results are presented to be used as a guidance for designing complex 3D structures via 4D printing of 2D structures. Helix structure, twisting structure, DNA-like structures, and functional gripper are designed to demonstrate the potential of direct FDM 4D printing for creating complex 3D structures from simple 2D structures with advantages over traditional manufacturing methods. It is shown that, by removing the need for a layer-by-layer stacking process to achieve a complex 3D shape, FDM can promote sustainability via 4D printing of autonomous 2D-to-3D shape transformer structures with lower materials, time, energy, and longer service life.

Item Type: Journal article
Publication Title: Advanced Engineering Materials
Creators: Hu, G. and Bodaghi, M.
Publisher: Wiley
Date: 1 July 2023
ISSN: 1438-1656
Identifiers:
NumberType
10.1002/adem.202300334DOI
1791725Other
Rights: This is an open access article under the terms of the Creative Commons Attribution License, which permits use, distribution and reproduction in any medium, provided the original work is properly cited.
Divisions: Schools > School of Science and Technology
Record created by: Jonathan Gallacher
Date Added: 17 Aug 2023 08:26
Last Modified: 17 Aug 2023 08:26
URI: https://irep.ntu.ac.uk/id/eprint/49578

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